Abstract. In this study, we experimentally investigate the variation of the phase matching condition of the high harmonic generation (HHG) process with pure argon gas and an argon-neon gas mixture. Phase-matched HHG is generated around the absorption edge of argon gas and then neon gas is added to the original argon gas. The pressure-dependent intensity of the harmonics produced by pure argon gas and the gas mixture is examined. We show that as more neon gas is added to the mixture, the phase matching of the higher order harmonics is less favourable than that of the lower order harmonics. Finally, the total phase mismatch at various gas mixture pressures is discussed. Our experimental results are in agreement with the theoretical calculation.

Key words: High harmonic generation, phase matching, nonlinear optics.